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Journal Articles

Development of a practical tritiated water monitor to supervise the discharge of treated water from Fukushima Daiichi Nuclear Power Plant

Sanada, Yukihisa; Oshikiri, Keisuke*; Kanno, Marina*; Abe, Tomohisa

Nuclear Instruments and Methods in Physics Research A, 1062, p.169208_1 - 169208_7, 2024/05

As part of the decommissioning work at the Fukushima Daiichi Nuclear Power Plant (FDNPP), the release of stored treated water began in 2023. In this study, we developed a practical tritium monitor to continuously monitor the concentration of tritiated water, as confirmed by batch sampling measurements at the FDNPP. The monitor is arranged with a flow cell detector comprising inexpensive plastic scintillator pellets and incorporating simultaneous measurements by three detectors, a veto detector, and lead shielding to reduce the influence of environmental $$gamma$$-rays. The system reached a detection limit of 911 Bq L-1 with a measurement time of 30 min, which is lower than the discharge standard for tritiated water of 1,500 Bq L-1. The system can also qualitatively distinguish the presence of disturbances due to interfering radionuclides other than tritium or background radiation using the $$beta$$-ray spectrum.

Journal Articles

In-operando distribution measurement of internal temperature and stress in lithium-ion battery

Hirano, Tatsumi*; Maeda, Takehiro*; Murata, Tetsuyuki*; Yamamoto, Takahiro*; Matsubara, Eiichiro*; Shobu, Takahisa; Shiro, Ayumi*; Yasuda, Ryo*; Takamatsu, Daiko*

SPring-8/SACLA Riyo Kenkyu Seikashu (Internet), 11(5), p.345 - 353, 2023/10

no abstracts in English

Journal Articles

Tritium inventory and its temporal variation in Fukushima Front Sea Area; Comparison between coastal and offshore tritium inventories and 1f treated water and operational target values for discharge per year

Machida, Masahiko; Iwata, Ayako; Yamada, Susumu; Otosaka, Shigeyoshi*; Kobayashi, Takuya; Funasaka, Hideyuki*; Morita, Takami*

Nihon Genshiryoku Gakkai Wabun Rombunshi (Internet), 22(1), p.12 - 24, 2023/01

We estimate inventory of tritium in two sea areas corresponding to coastal and offshore ones around Fukushima Daiichi Nuclear Power Plant (1F) based on the measurement results of sea-water tritium concentration monitored constantly from 2013 to Jan. 2021 by using Voronoi tessellation scheme. The obtained results show that the offshore area inventory and its temporal variation amount correspond to approximately 1/5 and 1/40 of that of the treated-water accumulated inside 1F, respectively. These results just suggest that the presence of tritium already included in sea-water as the background is non negligible in evaluating the environmental impact by releasing the accumulated treated-water into the sea region. We also estimate the offshore area inventory before 1F accident and find that it had exceeded over 1F stored inventory over about 30 years from 1960s to 1980s with approximately 4 times larger in the peak decade, 1960s. This fact means that we had already experienced more contaminated situation over 30 years in the past compared to the conservative case appeared by just releasing whole the present 1F inventory. Here, it should be also emphasized that the past contaminated situation was shared by the entire world. We further extend the estimation region into a wider region including an offshore area from Miyagi to Chiba prefectures and find that the area average inventory is now comparable to a half of the present 1F one. Finally, we estimate internal dose per year via ingesting fishes caught inside the area when 1F inventory is just added inside the area and kept for a year. The result indicates that it approximately corresponds to 1.0$$^-6$$ of the dose from natural radiation sources. From these estimation results, it is found that all the tritium inventory stored inside 1F never contribute to significant dose increment even when it is instantly released into the area.

Journal Articles

Basic study on tritium monitor using plastic scintillator for treated water discharge at Fukushima Daiichi Nuclear Power Plant

Sanada, Yukihisa; Abe, Tomohisa; Sasaki, Miyuki; Kanno, Marina*; Yamada, Tsutomu*; Nakasone, Takamasa*; Miyazaki, Nobuyuki*; Oshikiri, Keisuke*; Watabe, Hiroshi*

Journal of Nuclear Science and Technology, 10 Pages, 2023/00

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

The "treated water" from which the main radioactive materials were removed contains tritium, and stakeholders in Japan have been debating how to treat it. The amount of treated water stored in the facility has reached its limit, and the Japanese government has decided that the treatment method will be to discharge the water into the ocean by FY 2023 (FY: Fiscal Year). The present research developed a simple and practical tritium monitor for the Fukushima Daiichi Nuclear Power Station (FDNPS) tritiated water release. A simple and practical tritium monitor was developed for FDNPS tritiated water release based on thin plastic scintillator sheets. The developed devices were calibrated using standard tritium solutions and a method for calculating the minimum detectable activity. Fifteen 0.25 mm-thick scintillators can be placed in the 0.26 L flow cell where the sample water is fed, yielding an active surface area of 3,200 mm$$^{2}$$. The efficiency of tritiated water with full water is 0.000035 cps Bq$$^{-1}$$. The minimum detectable activity under simple shielding conditions was 7,800 Bq L$$^{-1}$$ (Measurement time was 3,600 s).

Journal Articles

Operando Br K-edge dispersive X-ray absorption fine structure analysis for Br$$^{-}$$/Br$$_{3}$$$$^{-}$$ redox mediator for Li-Air batteries

Ito, Kimihiko*; Matsumura, Daiju; Song, C.*; Kubo, Yoshimi*

ACS Energy Letters (Internet), 7(6), p.2024 - 2028, 2022/06

 Times Cited Count:2 Percentile:29.01(Chemistry, Physical)

Journal Articles

Estimation of temporal variation of discharged tritium from port of Fukushima Dai-ichi Nuclear Power Plant; Analysis of the temporal variation and comparison with released tritium from Japan and major nuclear facilities worldwide

Machida, Masahiko; Iwata, Ayako; Yamada, Susumu; Otosaka, Shigeyoshi*; Kobayashi, Takuya; Funasaka, Hideyuki*; Morita, Takami*

Nihon Genshiryoku Gakkai Wabun Rombunshi, 21(1), p.33 - 49, 2022/03

We estimate monthly discharge inventory of tritium from the port of Fukushima Daiichi Nuclear Power Plant (1F) from Jun 2013 to Mar 2020 by using the Voronoi tessellation scheme, following that the tritium monitoring inside the port has started since Jun 2013. As for the missing period from the initial month, Apr 2011 to May 2013, we calculate it by utilizing the concentration ratio of tritium to that of $$^{137}$$Cs in stagnant contaminant water during the initial direct discharged period to Jun 2011 and the discharge inventory correlation between tritium and $$^{137}$$Cs for the next-unknown continuously-discharged period up to May 2013. From the all- estimated results over 9 years, we find that the monthly discharge inventory sharply dropped just after closing the sea-side impermeable sea-wall in Oct. 2015 and subsequently coincided well with the sum of those of drainage and subdrain. By comparing the estimated results with those in the normal operation period before the accident, we point out that the discharge inventory from 1F port is not so large compared to those during the normal operation. Even the estimated one in year 2011 is found to be comparable to the maximum of operating pressurized water reactors discharging relatively large inventory in the order. In the nation level, the whole Japan domestic discharge inventory significantly decreased after the accident due to operation shutdown of most plants. Furthermore, 1F and even Japanese total discharge inventory are found to be entirely minor when comparing those of nuclear reprocessing plants and heavy-water reactors in world-wide level. From the above, we suggest that various scenarios can be openly discussed on the management in tritium stored inside 1F with help of the present estimated data and its comparison with the past discharge inventory.

Journal Articles

Microscopic dynamics of lithium diffusion in single crystal of the solid-state electrolyte La$$_{2/3-x}$$Li$$_{3x}$$TiO$$_{3}$$ (x = 0.13) studied by quasielastic neutron scattering

Matsuura, Masato*; Fujiwara, Yasuyuki*; Moriwake, Hiroki*; Ohara, Koji*; Kawakita, Yukinobu

Physical Review B, 104(9), p.094305_1 - 094305_7, 2021/09

 Times Cited Count:5 Percentile:44.86(Materials Science, Multidisciplinary)

Journal Articles

Correlated Li-ion migration in the superionic conductor Li$$_{10}$$GeP$$_{2}$$S$$_{12}$$

Yajima, Takeshi*; Hinuma, Yoyo*; Hori, Satoshi*; Iwasaki, Rui*; Kanno, Ryoji*; Ohara, Takashi; Nakao, Akiko*; Munakata, Koji*; Hiroi, Zenji*

Journal of Materials Chemistry A, 9(18), p.11278 - 11284, 2021/05

 Times Cited Count:19 Percentile:80.41(Chemistry, Physical)

Journal Articles

Experimental study of the $$Gamma_{p1}/Gamma_{p0}$$ ratios of resonance states in $$^{8}$$Be for deducing the $$^{7}$$Be($$n$$,$$p_{1}$$)$$^{7}$$Li$$^{*}$$ reaction rate relevant to the cosmological lithium problem

Iwasa, Naohito*; Ishikawa, Shunki*; Kubono, Shigeru*; Sakakibara, T.*; Kominato, Kazuya*; Nishio, Katsuhisa; Matsuda, Makoto; Hirose, Kentaro; Makii, Hiroyuki; Orlandi, R.; et al.

Physical Review C, 103(1), p.015801_1 - 015801_5, 2021/01

 Times Cited Count:1 Percentile:18.91(Physics, Nuclear)

JAEA Reports

Tritium removal of heavy water system and helium system in FUGEN

Takiya, Hiroaki; Kadowaki, Haruhiko; Matsushima, Akira; Matsuo, Hidehiko; Ishiyama, Masahiro; Aratani, Kenta; Tezuka, Masashi

JAEA-Technology 2020-001, 76 Pages, 2020/05

JAEA-Technology-2020-001.pdf:6.06MB

Advanced Thermal Reactor (ATR) FUGEN was operated for about 25 years, and now has been proceeding decommissioning after the approval of the decommissioning plan in Feb. 2008. The reactor, heavy water system and helium system are contaminated by tritium because of neutron absorption of heavy water, which is a moderator. Before dismantling these facilities, it is necessary to remove tritium from them for not only reducing the amount of tritium released to surrounding environment and the risk of internal exposure by tritium but also ensuring the workability. In first phase of decommissioning (Heavy Water and Other system Decontamination Period), tritium decontamination of the reactor, heavy water system and helium system started in 2008 and completed in 2018. This report shows the results of tritium decontamination of the reactor, heavy water system and helium system.

Journal Articles

Porous metal-organic frameworks containing reversible disulfide linkages as cathode materials for lithium-ion batteries

Shimizu, Takeshi*; Wang, H.*; Matsumura, Daiju; Mitsuhara, Kei*; Ota, Toshiaki*; Yoshikawa, Hirofumi*

ChemSusChem, 13(9), p.2256 - 2263, 2020/05

 Times Cited Count:24 Percentile:77.17(Chemistry, Multidisciplinary)

Journal Articles

Status of decommissioning of FUGEN Decommissioning Engineering Center

Takiya, Hiroaki; Aratani, Kenta; Awatani, Yuto; Ishiyama, Masahiro; Tezuka, Masashi; Mizui, Hiroyuki

Dekomisshoningu Giho, (59), p.2 - 12, 2019/03

FUGEN Decommissioning Engineering Center received the approval of the decommissioning program in 2008, and we have been progressing the decommissioning. The first phase of decommissioning (Heavy Water and Other system Decontamination Period) finished in May 2018, and FUGEN has entered into the second phase of decommissioning (Reactor Periphery Facilities Dismantling Period). This report outlines the results obtained in the first phase of decommissioning of FUGEN.

Journal Articles

In situ X-ray absorption fine structure studies of amorphous and crystalline polyoxovanadate cluster cathodes for lithium batteries

Wang, H.*; Idobe, Jin*; Matsumura, Daiju; Yoshikawa, Hirofumi*

Journal of Solid State Electrochemistry, 22(7), p.2067 - 2071, 2018/07

 Times Cited Count:15 Percentile:40.22(Electrochemistry)

Journal Articles

Theoretical model analysis of $$(d,xn)$$ reactions on $$^7$$Li at 25, 40, and 102 MeV

Sadamatsu, Hiroki*; Nakayama, Shinsuke; Watanabe, Yukinobu*; Iwamoto, Osamu; Ogata, Kazuyuki*

JAEA-Conf 2017-001, p.135 - 140, 2018/01

In recent years, the demand for intense neutron sources has been increasing in various applications such as nuclear transmutation of high-level radioactive waste and medical radioisotopes production. Deuteron accelerator-based neutron sources are promised as one of the candidates. Therefore, we have developed a code system dedicated for the deuteron-induced reactions, called DEURACS. In the present work, we focus on deuteron-induced neutron production from $$^7$$Li target. The calculated double differential cross sections for $$(d,xn)$$ reactions at incident energies of 25, 40, and 102 MeV are compared with the measured ones, and the applicability of DEURACS is discussed.

JAEA Reports

Verification of alternative dew point hygrometer for CV-LRT in Monju

Ichikawa, Shoichi; Chiba, Yusuke; Ono, Fumiyasu; Hatori, Masakazu; Kobayashi, Takanori; Uekura, Ryoichi; Hashiri, Nobuo*; Inuzuka, Taisuke*; Kitano, Hiroshi*; Abe, Hisashi*

JAEA-Research 2016-021, 32 Pages, 2017/02

JAEA-Research-2016-021.pdf:5.0MB

In order to reduce the influence on a plant schedule of the MONJU by the maintenance of dew point hygrometers, The JAEA examined a capacitance type dew point hygrometer as an alternative dew point hygrometer for a lithium-chloride type dew point hygrometer which had been used at the CV-LRT in the MONJU. As a result of comparing a capacitance type dew point hygrometer with a lithium-chloride type dew point hygrometer at the CV-LRT (Atmosphere: nitrogen, Testing time: 24 hours), there weren't significant difference between a capacitance type dew point hygrometer and a lithium-chloride type dew point hygrometer. As a result of comparing a capacitance dew point hygrometer with a high-mirror-surface type dew point hygrometer for long term verification (Atmosphere: air, Testing time: 24 months), the JAEA confirmed that a capacitance type dew point hygrometer satisfied the instrument specification ($$pm$$2.04$$^{circ}$$C) required by the JEAC4203-2008.

Journal Articles

Additional information to report on site tour of the Fukushima Daiichi Nuclear Power Station

Suto, Toshiyuki

Genshiryoku, hoshasen Bukaiho (Internet), (19), P. 15, 2016/12

The Tritiated Water Task Force under METI's Committee on Countermeasures for Contaminated Water Treatment for Fukushima Daiichi Nuclear Power Plant (1F) reported that the option of post-dilution offshore release could dispose the tritiated water at a smallest cost in the shortest amount of time. The amount of tritium in the contaminated water at 1F was compared with ones released from nuclear power plants and reprocessing plants as some help for grasping its level of magnitude.

Journal Articles

Report on site tour of the Fukushima Nuclear Power Station

Suto, Toshiyuki

Gijutsushi, 28(11), p.8 - 11, 2016/11

Five years have passed since the accident of the Fukushima Daiichi Nuclear Power Station. The Nuclear and Radiation section of the Institute of Professional Engineers hosted a site tour of the plant to make themselves sure what is going on in it and to disseminate information about it. The conditions of landscape during traveling between the gathering place and the plant, each reactor, contaminated water treatment, site, and work environment improvement will be reported.

Journal Articles

Nitrogen hot trap design and manufactures for lithium test loop in IFMIF/EVEDA project

Wakai, Eiichi; Watanabe, Kazuyoshi*; Ito, Yuzuru*; Suzuki, Akihiro*; Terai, Takayuki*; Yagi, Juro*; Kondo, Hiroo; Kanemura, Takuji; Furukawa, Tomohiro; Hirakawa, Yasushi; et al.

Plasma and Fusion Research (Internet), 11, p.2405112_1 - 2405112_4, 2016/11

BB2015-1982.pdf:2.03MB

Journal Articles

Study on pretreatment methods using a rapid combustion apparatus for the analyses of Organically Bound Tritium (OBT) in environmental samples

Manabe, Sachi; Matsubara, Natsumi; Saegusa, Jun; Takeishi, Minoru

KEK Proceedings 2016-8, p.281 - 285, 2016/10

no abstracts in English

Journal Articles

R-matrix analysis for the $$^8$$Be system and features in the p+$$^7$$Li reaction over resonance region

Kunieda, Satoshi

EPJ Web of Conferences, 122, p.08003_1 - 08003_13, 2016/06

The p+$$^7$$Li reaction is highly relevant to accelerator applications and fundamental physics. Therefore, those reaction cross-sections should be quantitatively known over the relevant energy range. However, in-depth theoretical/evaluation works have not necessarily been reported despite a number of experimental data which have been measured over the years. In this work, a multi-channel R-matrix analysis is carried out for $$^8$$Be system to know explicit natures in p+$$^7$$Li reaction over the resonance region. Present analysis reveals contribution from each $$J^{pi}$$ to the cross-sections and impact from direct process.

824 (Records 1-20 displayed on this page)